- Directed 2 actors to an Oscar nominated performance: Natalie Portman and Kristen Stewart.
- Son of politicians Hernán Larraín and Magdalena Matte.
- Graduated an all-boys private Catholic school: San Francisco de Asís in Las Condes, Santiago.
- Graduated from University of Arts, Science and Communication (aka UNIACC).
- Co-own production company - Fabula Productions.
- Brother of Hernán Larraín Matte, Juan de Dios Larraín, Magdalena, María José and Blanca.
- Began a relationship with actress Antonia Zegers in January 2006. They married on 9 December 2006, but separated in 2014.
- Father of Juana Larraín (b. March 2008) and Pascual Larraín (b. November 2011) with Antonia Zegers.
- Great-great-grandson of former Chile president Arturo Alessandri.
- Has also directed TV commercials for Latin America starring Valeria Mazza, Chayanne and Ricky Martin.
- Was a member of the jury at the Venice Film Festival in 2013.
- His movie No (2012) was Oscar-nominated for "Best Foreign Language Film".
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